A method for reactor synthesis based on process intensification principles and optimization of superstructure consisting of phenomenological modules

Zivkovic Luka A.; Nikacevic Nikola M.

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A method for reactor synthesis based on process intensification principles and optimization of superstructure consisting of phenomenological modules

机译：基于过程的反应器的方法合成强化原则和优化上层建筑组成的现象学模块

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A novel method for reaction synthesis is proposed. The method establishes strong interconnection between process intensification (PI) principles and process system engineering (PSE) techniques, which are used for problem formulation and optimization. The general aim is to demonstrate a potential for innovative solutions that combine both optimal reactor structure and its operational regime. The method consists of three stages: (I) Reaction Screening, in which phenomenological modules are defined; (II) Reaction System Superstructure and Mathematical Modeling in which modules (building blocks) are connected in a generic reactor superstructure; and (III) Optimization in which optimal structure and operational regime is derived, using techno-economical objective function and different optimization methods. The proposed method is demonstrated on a general example of two parallel endothermic reactions in liquid phase. The optimization results show that continuous steady-state reactor system outperforms fed-batch reactor and has similar performance as more complex periodically operated continuous reactor, and thus presents the optimal solution. (C) 2016 Institution of Chemical Engineers. Published by Elsevier B.V. All rights reserved.

机译：提出了反应合成的新方法。方法建立强大的互联过程强化(π)之间的原则和过程系统工程(PSE)技术,这是用于制定和问题优化。潜在的创新结合的解决方案这两个反应堆结构及其优化运营机制。阶段:(I)反应筛选,现象学模块定义;反应系统的上层建筑和数学建模模块(积木)连接在一个通用的反应堆上层建筑;和(3)优化的最优结构使用和操作制度,techno-economical目标函数和不同的优化方法。方法演示了在一个通用的例子两个平行的吸热反应液体阶段。连续稳态反应器系统优于馈料式反应堆,类似定期性能更复杂的操作连续反应器,从而提出最优解决方案。工程师。保留。

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来源
《Chemical Engineering Research & Design: Transactions of the Institution of Chemical Engineers》 |2016年第9期|189-205|共17页
作者
Zivkovic Luka A.; Nikacevic Nikola M.;
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作者单位

Univ Belgrade, Fac Technol & Met, Dept Chem Engn, Karnegijeva 4, Belgrade 11000, Serbia;

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原文格式 PDF
正文语种英语
中图分类
关键词
process systems; Process intensification; SuperstructuresReactorsProblem Formulation;

机译：过程系统;过程强化;SuperstructuresReactorsProblem配方;

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A method for reactor synthesis based on process intensification principles and optimization of superstructure consisting of phenomenological modules

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